CPET0026 CAM Detergents Cont Service (Wei Pan)

Projects

Notes

Most of these experiments were canceled. We tested the transmission signal from attrited layers and compared them to R-9-9

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58B attrited (Fresh DeH-15 2823)

~9 mg of sample pressed into 4 barrel

step 1

09aug_PtL3.003

As Rec, RT in He

RT

air

Pt L3 xanes

edge step 0.01

33656-58H attrited (repeated treatement on DeH-15 2883 as 33636-58F)

~161 mg of sample pressed into 4 barrel

step 1

09aug_PtL3.004

As Rec, RT in He

RT

air

Pt L3 xanes

edge step 0.3, sample too thick due to Sn

R-9-9(reference sample Pt only 0.375 wt% Pt)

~50 mg of sample pressed into 4 barrel

step 1

09aug_PtL3.005

As Rec, RT in He

RT

air

Pt L3 xanes

edge step 0.06

Whole Pills, Ground

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58B (Fresh DeH-15 2823)

~XXXmg of Whole Pills Ground

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time =5.0hrs

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58F (DeH-15 2883; wet reduced @ 200c, 4000ppm H2O/H2, 116hr)

~XXXmg of Whole Pills Ground

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time = 5.0hr

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58H (Repeated treatment on DeH-15 2883 as 33656-58F)

~XXXmg of Whole Pills Ground

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time =5.0hrs

Attrited Layers

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58B (

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58B (Fresh DeH-15 2823)

~XXXmg of Whole Pills Ground

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

)

~XXXmg of Attrited Layer

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time =5.0 hrs

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58D (DeH-15 2842; Wet reduced @ 290C, 4000ppm H2O/H2, 116hr)

~XXXmg of Attrited Layer

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time 5.0 hrs

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58E (DeH-15 2883; wet reduced @ 200C, 620ppm H2O/H2, 116hr)

~XXXmg of Attrited Layer

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time =5.0 hrs

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58F (DeH-15 2883; wet reduced @ 200C, 4000 ppm H2O/H2, 116hr)

~XXXmg of Attrited Layer

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (0.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time = 5.0 hrs

#

filename

description

Temp

Gas

EXAFS/XANES

DONE

PIC

33656-58H (Repeated treatment DeH-15 2883 as 33656-58F)

~XXXmg of Attrited Layer

step 1 (0.25)

09aug_PtL3.xxx-xxx

As Rec, RT in He

RT

100%He

PtL3 Exafs

step 2

Ramp to 450C in H00% H2 @ 5C/min. 30 min Dwell

step 3 (2.0)

09aug_PtL3.xxx-xxx

PtL3 Xanes during TPR

RT to 450

100% H2

PtL3-Xanes

step 4 (0.5)

Cool to RT in H2

step 5 (1.0)

09aug_PtL3.xxx-xxx

PtL3 After reduction. RT in H2

RT

100% H2

PtL3 Exafs

step 6 (0.25)

09aug_PtL2.xxx-xxx

PtL2 Xanes after reduction. RT in H2

RT

100% H2

PtL2 XANES

step 7

Ramp to 350C @ 5C/min in 100% He

step 8 (1.0)

09aug_PtL2.xxx-xxx

PtL2 Xanes During ramp to 350c in He

RT to 350C

100% He

PtL2 XANES

Time =5.0hrs

UOP/10BM.2009.08.CAM (last edited 2009-10-09 19:50:57 by localhost)